Both devices must be on the same local network, and Control by mobile apps must be turned on in Roku's system settings.
To explore advanced ways to connect your devices, let me know: Is your currently connected to the internet? Do you know your Roku's current IP address ? Online Remote for Roku - Free TV Remote Control
Because browser-based remotes utilize your local network, your Chromebook and Roku device must be properly connected. Step 1: Connect to the Same Wi-Fi Network
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